This was written by Toto keyboard player David Paich and drummer Jeff Porcaro; Paich also sang lead. The song is about a girl who goes to Catholic school, but has a wild streak. In our interview with Paich, he said that his sister and her friends went to Catholic schools and provided inspiration for the track. "That's an amalgamation of a couple of my sister's girlfriends that I rolled into one girl, Holyanna," he said.
Note the religious imagery in the song title: Holyanna.
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